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Sarkomycin Synthesis Essay

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  • Total Synthesis of (−)-Nahuoic Acid Ci (Bii)

    Journal of the American Chemical Society

    Liu, Deng, and Smith

    2017139 (39), pp 13668–13671

    Abstract: A convergent total synthesis of (−)-nahuoic acid Ci(Bii) (3), a novel cis-decalin polyketide, has been achieved. Key synthetic transformations include Type II Anion Relay Chemistry (ARC) to construct the polyol chain, a Ti-catalyzed asymmetric Diels–Alder ...

    Abstract | Full Text HTML | PDF w/ Links | Hi-Res PDF

  • Total Synthesis of (+)-Pleuromutilin

    Journal of the American Chemical Society

    Farney, Feng, Schäfers, and Reisman

    2018140 (4), pp 1267–1270

    Abstract: An 18-step synthesis of the antibiotic (+)-pleuromutilin is disclosed. The key steps of the synthesis include a highly stereoselective SmI2-mediated cyclization to establish the eight-membered ring and a stereospecific transannular [1,5]-hydrogen atom ...

    Abstract | Full Text HTML | PDF w/ Links | Hi-Res PDF

  • Total Synthesis of (−)-Himalensine A

    Journal of the American Chemical Society

    Shi, Michaelides, Darses, Jakubec, Nguyen, Paton, and Dixon

    2017139 (49), pp 17755–17758

    Abstract: The first enantioselective synthesis of (−)-himalensine A has been achieved in 22 steps. The synthesis was enabled by a novel catalytic, enantioselective prototropic shift/furan Diels–Alder (IMDAF) cascade to construct the ACD tricyclic core. A reductive ...

    Abstract | Full Text HTML | PDF w/ Links | Hi-Res PDF

  • Total Synthesis of Longeracinphyllin A

    Journal of the American Chemical Society

    Li, Zhang, Zhang, Chen, and Li

    2017139 (42), pp 14893–14896

    Abstract: The first and asymmetric total synthesis of longeracinphyllin A, a hexacyclic Daphniphyllum alkaloid, has been accomplished. A tetracyclic intermediate was prepared through silver-catalyzed alkyne cyclization and Luche radical cyclization. A phosphine-...

    Abstract | Full Text HTML | PDF w/ Links | Hi-Res PDF

  • Total Syntheses of (−)-Majucin and (−)-Jiadifenoxolane A, Complex Majucin-Type Illicium Sesquiterpenes

    Journal of the American Chemical Society

    Condakes, Hung, Harwood, and Maimone

    2017139 (49), pp 17783–17786

    Abstract: We report the first chemical syntheses of both (−)-majucin and (−)-jiadifenoxolane A via 10 net oxidations from the ubiquitous terpene (+)-cedrol. Additionally, this approach allows for access to other majucin-type sesquiterpenes, like (−)-jiadifenolide, (...

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  • Enantioselective Total Syntheses of (+)-Hippolachnin A, (+)-Gracilioether A, (−)-Gracilioether E, and (−)-Gracilioether F

    Journal of the American Chemical Society

    Li, Zhao, Peuronen, Rissanen, Enders, and Tang

    2018140 (5), pp 1937–1944

    Abstract: The Plakortin polyketides represent a structurally and biologically fascinating class of marine natural products. Herein, we report a unified strategy that enables the divergent syntheses of various Plakortin polyketides with high step-economy and overall ...

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  • Finally done! i have to be up in 2 hrs to volunteer @ berkeley kite festival. is it worth sleeping? i'll just work on my research paper.

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